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Quick answer 60-second read Canonicalises to Who vs. Whom

Is it "who should I call" or "whom should I call"?

Strictly, "whom should I call" — the caller is doing the calling to someone.

A little morei

You would call him, not he, which means the object form whom is correct. "Who should I call" is common in speech and rarely sounds wrong. Edited prose still prefers "whom."

The full entryii

Usage
Who vs. Whom

Subject versus object — the pronoun doing it versus the pronoun it happens to.

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